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15 N spin–lattice relaxation dynamics in metronidazole- 15 N 3 and metronidazole- 15 N 2 isotopologues are studied for rational design of 15 N-enriched biomolecules for signal amplification by reversible exchange in microtesla fields. 15 N relaxation dynamics mapping reveals the deleterious effects of interactions with the polarization transfer catalyst and a quadrupolar 14 N nucleus within the spin-relayed 15 N– 15 N network.more » « less
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Coffey, Aaron M. ; Shchepin, Roman V. ; Truong, Milton L. ; Wilkens, Ken ; Pham, Wellington ; Chekmenev, Eduard Y. ( , Analytical Chemistry)
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Shchepin, Roman V. ; Birchall, Jonathan R. ; Chukanov, Nikita V. ; Kovtunov, Kirill V. ; Koptyug, Igor V. ; Theis, Thomas ; Warren, Warren S. ; Gelovani, Juri G. ; Goodson, Boyd M. ; Shokouhi, Sepideh ; et al ( , Chemistry – A European Journal)